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Three types of\nchemically homogeneous cellulose samples are used as surrogates that\nrepresent supermicron and submicron ice-nucleating plant structural\npolymers. These samples include microcrystalline cellulose (MCC), fibrous\ncellulose (FC) and nanocrystalline cellulose (NCC). Our immersion freezing\ndataset includes data from various ice nucleation measurement techniques\navailable at 17 different institutions, including nine dry dispersion\nand 11 aqueous suspension techniques. With a total of 20 methods, we\nperformed systematic accuracy and precision analysis of measurements from\nall 20 measurement techniques by evaluating T-binned (1??C)\ndata over a wide T range (?36??C?\u0026lt;T\u0026lt;-4??C). Specifically, we intercompared the geometric surface\narea-based ice nucleation active surface site (INAS) density data derived from\nour measurements as a function of T, ns,geo(T). 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  1. 防災科研関係論文

A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water

https://nied-repo.bosai.go.jp/records/5895
https://nied-repo.bosai.go.jp/records/5895
e5052634-24a0-4522-84d5-f077203a162e
Item type researchmap(1)
公開日 2023-03-30
タイトル
言語 en
タイトル A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water
言語
言語 eng
著者 Naruki Hiranuma

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en Naruki Hiranuma

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Kouji Adachi

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en Kouji Adachi

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David M. Bell

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en David M. Bell

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Franco Belosi

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en Franco Belosi

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Hassan Beydoun

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en Hassan Beydoun

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Bhaskar Bhaduri

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en Bhaskar Bhaduri

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Heinz Bingemer

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Carsten Budke

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Hans-Christian Clemen

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Franz Conen

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Kimberly M. Cory

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Joachim Curtius

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en Joachim Curtius

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Paul J. DeMott

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en Paul J. DeMott

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Oliver Eppers

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en Oliver Eppers

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Sarah Grawe

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en Sarah Grawe

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Susan Hartmann

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Nadine Hoffmann

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Kristina Hohler

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Evelyn Jantsch

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en Evelyn Jantsch

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Alexei Kiselev

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Thomas Koop

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Gourihar Kulkarni

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en Gourihar Kulkarni

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Amelie Mayer

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Masataka Murakami

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Benjamin J. Murray

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Alessia Nicosia

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Markus D. Petters

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Matteo Piazza

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en Matteo Piazza

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Michael Polen

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Naama Reicher

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Yinon Rudich

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Atsushi Saito

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Gianni Santachiara

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Thea Schiebel

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Gregg P. Schill

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Johannes Schneider

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Lior Segev

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Emiliano Stopelli

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Ryan C. Sullivan

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Kaitlyn Suski

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Miklos Szakall

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Takuya Tajiri

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Hans Taylor

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Yutaka Tobo

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Romy Ullrich

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Daniel Weber

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Heike Wex

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Thomas F. Whale

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Craig L. Whiteside

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Katsuya Yamashita

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Alla Zelenyuk

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Ottmar Mohler

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抄録
内容記述タイプ Other
内容記述 Abstract. We present the laboratory results of immersion freezing efficiencies of
cellulose particles at supercooled temperature (T) conditions. Three types of
chemically homogeneous cellulose samples are used as surrogates that
represent supermicron and submicron ice-nucleating plant structural
polymers. These samples include microcrystalline cellulose (MCC), fibrous
cellulose (FC) and nanocrystalline cellulose (NCC). Our immersion freezing
dataset includes data from various ice nucleation measurement techniques
available at 17 different institutions, including nine dry dispersion
and 11 aqueous suspension techniques. With a total of 20 methods, we
performed systematic accuracy and precision analysis of measurements from
all 20 measurement techniques by evaluating T-binned (1??C)
data over a wide T range (?36??C?<T<-4??C). Specifically, we intercompared the geometric surface
area-based ice nucleation active surface site (INAS) density data derived from
our measurements as a function of T, ns,geo(T). Additionally, we also
compared the ns,geo(T) values and the freezing spectral slope parameter
(Δlog(ns,geo)/ΔT) from our measurements to previous
literature results. Results show all three cellulose materials are
reasonably ice active. The freezing efficiencies of NCC samples agree
reasonably well, whereas the diversity for the other two samples spans
??10??C. Despite given uncertainties within each
instrument technique, the overall trend of the ns,geo(T) spectrum traced
by the T-binned average of measurements suggests that predominantly
supermicron-sized cellulose particles (MCC and FC) generally act as more
efficient ice-nucleating particles (INPs) than NCC with about 1 order of
magnitude higher ns,geo(T).
言語 en
書誌情報 en : Atmospheric Chemistry and Physics

巻 19, 号 7, p. 4823-4849, 発行日 2019-04-10
出版者
言語 en
出版者 Copernicus GmbH
ISSN
収録物識別子タイプ EISSN
収録物識別子 1680-7324
DOI
関連識別子 10.5194/acp-19-4823-2019
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